Nano Science and Technology Institute
Nanotech 2003 Vol. 1
Nanotech 2003 Vol. 1
Technical Proceedings of the 2003 Nanotechnology Conference and Trade Show, Volume 1
Chapter 9: Micro Fluidics

CFD-based Optimization of Gas/Liquid Microreactors with Droplet and Bubble Transport

Authors:S. Hardt, H. Pennemann and F. Jiang
Affilation:Institute of Microtechnology Mainz, DE
Pages:254 - 257
Keywords:microreactors, free-surface flow, surface-directed flow, CFD
Abstract:Microreactors offer unique opportunities for the control of process parameters unparalleled by macroscopic equipment. A new gas/liquid microreactor is proposed allowing for fast mass transfer and small concentration gradients as well as a very narrow residence time distribution. The reactor should be ideally suited for the screening of gas/liquid reactions and allow to measure kinetic data with a high degree of accuracy. The reaction chamber consists of an arrangement of two parallel plates with hydrophilic strips along which droplets are transported by a gas stream. Besides propelling the droplets, the gas is used as a carrier for the species to be transferred to the liquid phase. In order to simulate droplet formation and transport, a 3D FVM volume tracking technique is employed. It is shown that for comparatively small gas velocities, the droplets are driven by the flow but are not disrupted.Droplets of suitable size can be created by nozzles directing liquid flow perpendicular to the plates. Based on the design concepts supported by the CFD simulations, a prototype reactor was fabricated from glass, thus allowing to follow droplet formation and transport with a CCD camera. First experimental results obtained with a corresponding set-up are presented and compared with the simulations.
CFD-based Optimization of Gas/Liquid Microreactors with Droplet and Bubble TransportView PDF of paper
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